Vladan Vuletic
Assistant Professor, Department of Physics
Varian Building
382 Via Pueblo Mall
Stanford, CA 94305-4060
office Rm. 238, labs 243, 244
phone (650) 723-4233
fax (650) 723-9173
vladan.vuletic@stanford.edu, vladan2@stanford.edu
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lab |
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| Vuletic, Vladan |
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vladan.vuletic@stanford.edu
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| Black, Adam |
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adam.black@stanford.edu
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| Chan, Hilton |
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chanhw@stanford.edu
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| Chin, Cheng | Postdoc |
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cchin@stanford.edu
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| Lin, Yu-ju | Research Assistant |
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yjlin@stanford.edu
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| Teper, Igor |
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teper@stanford.edu
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New laser cooling methods for atoms, ions or molecules: Cavity Doppler cooling and cavity sideband cooling by coherent scattering
Laser cooling of atoms has not only supplied the basis
for the control and manipulation of matter at the quantum limit, e.g. in
form of Bose-Einstein condensation, but has also resulted in a number of
important applications and devices, many of which are tied to precision
measurements and atomic clocks. However, laser cooling has so far been
limited to atoms with a particular internal structure, and the cooling
of molecules or even of atoms with a complicated level scheme has so far
not been possible. If we could learn how to cool, trap and manipulate larger
molecules in the same way as atoms, this would open the door for important
developments in chemistry and possibly even in biology.
Doppler cooling [1] is the dominant
laser cooling mechanism at all but the lowest temperatures. In Doppler
cooling counterpropagating laser beams are tuned to the red of a closed
transition between an atomic ground and an atomic excited state. An atom
that is moving towards a laser beam will experience photons that are blue-shifted
into resonance with the atomic transition, while photons from a beam propagating
in the same direction as the atom will be red-shifted further out of resonance.
The momentum transfer associated with the preferred absorption of photons
from the counterpropagating beam leads to slowing and cooling of the atoms,
while the randomly emitted photons on average do not contribute to the
force. The net effect is cooling to temperatures in the millikelvin to
microkelvin range, corresponding to atomic velocities in the range of a
few millimeters to a few centimeters per second.
This principle behind laser cooling
also entails its limitation. Since the momentum “kick” associated with
each photon absorption event is much smaller than the momentum of a thermal
atom, a larger number of absorption-emission events (on the order of thousand
or more) is required to significantly change the atom’s velocity. Therefore
laser cooling has only been demonstrated with atoms that can be optically
cycled many times back to their initial ground state. However, most atoms
(and all molecules) have multiple ground states to which the excited state
can decay. Once the atom reaches a different ground state, the laser no
longer has the correct detuning relative to the atomic transition, and
the cooling stops. In particular, molecules have many vibrational and rotational
levels, and consequently no laser cooling of molecules has been demonstrated.
The novel proposed method [2,3] is
based on coherent scattering, rather than on spontaneous emission from
an excited state. Coherent scattering dominates when the laser is far detuned
from atomic or molecular transitions and when its intensity is not too
large. Coherent scattering is generic to all polarizable particles, independent
of their internal structure, and describes the emission of radiation by
an oscillating atomic dipole that is driven by an external (classical)
electric field. The basic idea behind the proposed technique is that energy
is conserved in the scattering process, and that therefore events where
the scattered photon carries away a larger energy than the incident-photon
energy are accompanied by a corresponding reduction of the atom’s energy.
Such scattering events can be enhanced in an optical resonator that is
tuned to be resonant with a frequency that is higher than that of the incident
light. The new cooling mechanism depends only on the finesse (i.e. on the
reflectivity of the cavity mirrors) and on the detuning of the photons
relative to the cavity resonance, while it is independent of the detuning
relative to atomic transitions. Therefore this new technique should be
generic and be applicable to any sort of material. The target can be an
atom in different ground states, a molecule in different rotational and
vibrational states, or possibly even a scattering center (impurity) inside
a solid. The only requirement is that at the given intensity and laser
frequency the emission rate by the scatterer is large enough to produce
efficient cooling. The cooling power is given by the product of the scattering
rate and the energy difference between the incident and the scattered photon
[2].
We are currently preparing a proof-of-principle
experiment where cesium atoms are cooled with the new technique using light
that is far detuned from any atomic transitions. Since the new technique
is closely related to Doppler cooling [2,4], the cooling limit will be
given by the Doppler limit for the cavity linewidth, i.e. the temperature
at which the thermal energy of the atoms equals the energy that corresponds
to the linewidth of the resonator. Therefore temperatures near the recoil
limit should be attainable with low loss mirror substrates, independent
of the atomic structure or atomic linewidth.
[1] T.W. Hänsch and A.L. Schawlow, Opt.
Commun. 13, 68 (1975).
[2] V. Vuletic and S. Chu, Phys. Rev. Lett.
84,
3787 (2000).
[3] P. Horak, G. Hechenblaikner, K.M. Gheri,
H. Stecher, and H. Ritsch, Phys. Rev. Lett. 79, 4974 (1997).
[4] V. Vuletic, H. W. Chan, and A. T. Black,
Phys. Rev. A 64, 033405 (2001).
New laser cooling methods
for atoms, ions or molecules: Cavity cooling by coherent scattering
Laser cooling: Degenerate Raman
sideband cooling
Cold collisions of cesium atoms,
Feshbach resonances
Laser spectroscopy
Laser design
Other subjects